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Because all Incantors output the same basic signals, musicality is generally the same. Read the previous description of the original Speak & Spell s output for insights, in Project 1. I especially like the bent Speak & Read s ability to string words together into amusing sentences. Don t be surprised if your model says Let s smell the scissors s more.

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Equations 3-96 through 3-98 show a signi cant characteristic of radical chain polymerizations. The kinetic chain length is inversely dependent on the radical concentration or the polymerization rate. This is of great practical signi cance any attempt to increase the polymerization rate by increasing the radical concentration comes at the expense of producing smaller polymer molecules. The kinetic chain length at constant polymerization rate is a characteristic of the particular monomer and independent of the method of initiation. Thus, for any monomer, n is independent of whether the polymerization is initiated by thermal, redox, or photochemical means, whether initiators are used, or of the particular initiator used, if [R ] or Rp is the same. The general relationship between the degree of polymerization and the kinetic chain length is

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They were born of the government s desperate need for cash to carry on the war with France In 1692 the Parliament provided new duties on beer and other liquors to be set aside as security for a long-term loan of 1 million in the form of life annuities which would pay 10% until 1700 and thereafter 7% plus tontine benefits to long survivors (351) The creditors risk seemed considerable because William s regime was contested; if the Stuart Kings returned, they would repudiate the debts of William s government In 1693 another long-term loan of 1 million was floated, secured by a duty on salt, at 10% interest for 16 years plus lottery benefits, which brought the cost of the loan up.

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Although experimental data are not available for all monomers, most polymer radicals appear to terminate predominately or entirely by coupling (except where chain transfer predominates). Studies with small, aliphatic radicals clearly predict this tendency [Tedder, 1974]. However, varying extents of disproportionation are observed depending on the reaction system. Disproportionation increases when the propagating radical is sterically hindered or has many b-hydrogens available for transfer. Thus, whereas styrene, methyl acrylate, and acrylonitrile undergo termination almost exclusively by coupling, methyl methacrylate undergoes termination by a combination of coupling and disproportionation [Ayrey et al., 1977; Bamford, 1988; Bonta et al., 1976; Hensley et al., 1995]. Increased temperature increases the extent of disproportionation, with the most signi cant effect for sterically hindered radicals. The extent of disproportionation in methyl methacrylate increases from 67% at 25 C to 80% at 80 C [Bamford et al.,1969b]. There appears to be a tendency toward disproportionation for highly reactive radicals such as those in vinyl acetate and ethylene

polymerizations. However, the effect is relatively small as the extent of disproportionation in these two polymerizations is no greater than 10% at most [Bamford et al., 1969a,b].

In many polymerization systems the polymer molecular weight is observed to be lower than predicted on the basis of the experimentally observed extents of termination by coupling and disproportionation. This effect is due to the premature termination of a growing polymer by the transfer of a hydrogen or other atom or species to it from some compound present in the system the monomer, initiator, or solvent, as the case may be. These radical displacement reactions are termed chain-transfer reactions and may be depicted as

to 14% (352) This type of finance was costly and unsatisfactory The provinces of Holland were borrowing at 3 4%, and did not have to pledge specific revenues In 1694 another large war loan was required by the government This time a momentous expedient was devised As is usual with such innovations, doubts, fears, and prejudices were resolved by the acute national need and the uninviting character of the alternatives The Parliament passed an ambiguously worded bill to impose a new duty on tonnage for the benefit of such persons as should advance money toward carrying on the war.

Clearer sounding than any model before, the Speak & Math is also the most difficult of the later models to find (see Figure 17-1).

3-102

where XA may be monomer, initiator, solvent, or other substance and X is the atom or species transferred. Chain transfer to initiator was referred to earlier as induced initiator decomposition (Sec. 3-4g-1). The rate of a chain-transfer reaction is given by